Publications

An important goal of modern condensed-matter physics involves the search for states of matter with emergent properties and desirable functionalities. Although the tools for material design remain relatively limited, notable advances have been recently achieved by controlling interactions at heterointerfaces, precise alignment of low-dimensional materials and the use of extreme pressures. Here we highlight a paradigm based on controlling light--matter interactions, which provides a way to manipulate and synthesize strongly correlated quantum matter. We consider the case in which both electron--electron and electron--photon interactions are strong and give rise to a variety of phenomena. Photon-mediated superconductivity, cavity fractional quantum Hall physics and optically driven topological phenomena in low dimensions are among the frontiers discussed in this Perspective, which highlights a field that we term here `strongly correlated electron--photon science'.

We explore pump-probe high harmonic generation (HHG) from monolayer hexagonal-Boron-Nitride, where a terahertz pump excites coherent optical phonons that are subsequently probed by an intense infrared pulse that drives HHG. We find, through state-of-the-art ab-initio calculations, that the structure of the emission spectrum is attenuated by the presence of coherent phonons, and is no longer comprised of discrete harmonic orders, but rather of a continuous emission in the plateau region. The HHG yield strongly oscillates as a function of the pump-probe delay, corresponding to ultrafast changes in the lattice such as bond compression or stretching. We further show that in the regime where the excited phonon period and the pulse duration are of the same order of magnitude, the HHG process becomes sensitive to the carrier-envelope-phase (CEP) of the driving field, even though the pulse duration is so long that no such sensitivity is observed in the absence of coherent phonons. The degree of CEP sensitivity vs. pump-probe delay is shown to be a highly selective measure for instantaneous structural changes in the lattice, providing a new approach for ultrafast multi-dimensional HHG-spectroscopy. Remarkably, the obtained temporal resolution for phonon dynamics is 1 femtosecond, which is much shorter than the probe pulse duration because of the inherent sub-cycle contrast mechanism. Our work paves the way towards novel routes of probing phonons and ultrafast material structural changes and provides a mechanism for controlling the high harmonic response.

We study the consequences of the approximately trigonal (D

High harmonic generation (HHG) takes place in all phases of matter. In gaseous atomic and molecular media, it has been extensively studied and is very well-understood. In solids research is ongoing, but a consensus is forming for the dominant microscopic HHG mechanisms. In liquids on the other hand, no established theory yet exit and approaches developed for gases and solids are generally inapplicable, hindering our current understanding. We develop here a powerful and reliable ab-initio cluster-based approach for describing the nonlinear interactions between isotropic bulk liquids and intense laser pulses. The scheme is based on time-dependent density functional theory and utilizes several approximations that make it feasible yet accurate in realistic systems. We demonstrate our approach with HHG calculations in water, ammonia, and methane liquids, and compare the characteristic response of polar and non-polar liquids. We identify unique features in the HHG spectra of liquid methane that could be utilized for ultrafast spectroscopy of its chemical and physical properties: (i) a structural minima at 15-17eV, and (ii) a well-like shape in the perturbative region that is reminiscent of a shape resonance. Our results pave the way to accessible calculations of HHG in liquids and illustrate the unique nonlinear nature of liquid systems.

Many-body interactions between quasiparticles (electrons, excitons, and phonons) have led to the emergence of new complex correlated states and are at the core of condensed matter physics and material science. In low-dimensional materials, unique electronic properties for these correlated states could significantly affect their optical properties. Herein, combining photoluminescence, optical reflection measurements and theoretical calculations, we demonstrate an unconventional excitonic state and its bound phonon sideband in layered silicon diphosphide (SiP

Many materials exhibit phase transitions at which both the electronic properties and the crystal structure change. Some authors have argued that the change in electronic order is primary, with the lattice distortion a relatively minor side-effect, and others have argued that the lattice distortions play an essential role in the energetics of the transition. In this paper, we introduce a formalism that resolves this long-standing problem. The methodology works with any electronic structure method that produces solutions of the equation of state determining the electronic order parameter as a function of lattice distortion. We use the formalism to settle the question of the physics of the metal--insulator transitions in the rare-earth perovskite nickelates (RNiO3) and Ruddlesden--Popper calcium ruthenates (Ca2RuO4) in bulk, heterostructure, and epitaxially strained thin film forms, finding that electron-lattice coupling is key to stabilizing the insulating state in both classes of materials.

Stellar streams in the Galactic halo are useful probes of the assembly of galaxies like the Milky Way. Many tidal stellar streams that have been found in recent years are accompanied by a known progenitor globular cluster or dwarf galaxy. However, the Orphan--Chenab (OC) stream is one case where a relatively narrow stream of stars has been found without a known progenitor. In an effort to find the parent of the OC stream, we use astrometry from the early third data release of ESA's Gaia mission (Gaia EDR3) and radial velocity information from the SDSS-IV APOGEE survey to find up to 13 stars that are likely members of the OC stream. We use the APOGEE survey to study the chemical nature (for up to 13 stars) of the OC stream in the α (O, Mg, Ca, Si, Ti, S), odd-Z (Al, K, V), Fe-peak (Fe, Ni, Mn, Co, Cr) and neutron capture (Ce) elemental groups. We find that the stars that make up the OC stream are not consistent with a mono-metallic population and have a median metallicity of --1.92~dex with a dispersion of 0.28 dex. Our results also indicate that the α-elements are depleted compared to the known Milky Way populations and that its [Mg/Al] abundance ratio is not consistent with second generation stars from globular clusters. The detailed chemical pattern of these stars indicates that the OC stream progenitor is very likely to be a dwarf spheroidal galaxy with a mass of ~106 M⊙.

The cytoskeleton -- a collection of polymeric filaments, molecular motors, and crosslinkers -- is a foundational example of active matter, and in the cell assembles into organelles that guide basic biological functions. Simulation of cytoskeletal assemblies is an important tool for modeling cellular processes and understanding their surprising material properties. Here we present aLENS, a novel computational framework to surmount the limits of conventional simulation methods. We model molecular motors with crosslinking kinetics that adhere to a thermodynamic energy landscape, and integrate the system dynamics while efficiently and stably enforcing hard-body repulsion between filaments -- molecular potentials are entirely avoided in imposing steric constraints. Utilizing parallel computing, we simulate different mixtures of tens to hundreds of thousands of cytoskeletal filaments and crosslinking motors, recapitulating self-emergent phenomena such as bundle formation and buckling, and elucidating how motor type, thermal fluctuations, internal stresses, and confinement determine the evolution of active matter aggregates.

The gravitational redshift induced by stellar surface gravity is notoriously difficult to measure for non-degenerate stars, since its amplitude is small in comparison with the typical Doppler shift induced by stellar radial velocity. In this study, we make use of the large observational data set of the Gaia mission to achieve a significant reduction of noise caused by these random stellar motions. By measuring the differences in velocities between the components of pairs of co-moving stars and wide binaries, we are able to statistically measure the combined effects of gravitational redshift and convective blueshifting of spectral lines, and nullify the effect of the peculiar motions of the stars. For the subset of stars considered in this study, we find a positive correlation between the observed differences in Gaia radial velocities and the differences in surface gravity and convective blueshift inferred from effective temperature and luminosity measurements. The results rule out a null signal at the 5σ level for our full data-set. Additionally, we study the sub-dominant effects of binary motion, and possible systematic errors in radial velocity measurements within Gaia. Results from the technique presented in this study are expected to improve significantly with data from the next Gaia data release. Such improvements could be used to constrain the mass-luminosity relation and stellar models which predict the magnitude of convective blueshift.

The abundance of bright galaxies at z>8 can provide key constraints on models of galaxy formation and evolution, as the predicted abundance varies greatly when different physical prescriptions for gas cooling and star formation are implemented. We present the results of a search for bright z=9-10 galaxies selected from pure-parallel Hubble Space Telescope imaging programs. We include 132 fields observed as part of the Brightest of Reionizing Galaxies survey, the Hubble Infrared Pure Parallel Imaging Extragalactic Survey, and the WFC3 Infrared Spectroscopic Parallel survey. These observations cover a total of 620 sq. arcmin, about 70% of which is also covered with Spitzer Space Telescope infrared imaging. We identify thirteen candidate galaxies in the range 8.3<z<11 with 24.5 < m_H < 26.5 (-22.9 < M_UV < -21.2). This sample capitalizes on the uncorrelated nature of pure parallel observations to overcome cosmic variance and leverages a full multi-wavelength selection process to minimize contamination without sacrificing completeness. We perform detailed completeness and contamination analyses, and present measurements of the bright end of the UV luminosity function using a pseudo-binning technique. We find a number density consistent with results from Finkelstein et al. (2022) and other searches in HST parallel fields. These bright candidates likely reside in overdensities, potentially representing some of the earliest sites of cosmic reionization. These new candidates are excellent targets for follow-up with JWST, and four of them will be observed with the NIRSpec prism in Cycle 1.