2573 Publications

Quantum feedback at the solid-liquid interface: flow-induced electronic current and negative friction

Baptiste Coquinot, Lydéric Bocquet, N. Kavokine
An electronic current driven through a conductor can induce a current in another conductor through the famous Coulomb drag effect. Similar phenomena have been reported at the interface between a moving fluid and a conductor, but their interpretation has remained elusive. Here, we develop a quantum-mechanical theory of the intertwined fluid and electronic flows, taking advantage of the non-equilibrium Keldysh framework. We predict that a globally neutral liquid can generate an electronic current in the solid wall along which it flows. This hydrodynamic Coulomb drag originates from both the Coulomb interactions between the liquid's charge fluctuations and the solid's charge carriers, and the liquid-electron interaction mediated by the solid's phonons. We derive explicitly the Coulomb drag current in terms of the solid's electronic and phononic properties, as well as the liquid's dielectric response, a result which quantitatively agrees with recent experiments at the liquid-graphene interface. Furthermore, we show that the current generation counteracts momentum transfer from the liquid to the solid, leading to a reduction of the hydrodynamic friction coefficient through a quantum feedback mechanism. Our results provide a roadmap for controlling nanoscale liquid flows at the quantum level, and suggest strategies for designing materials with low hydrodynamic friction.
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Interaction confinement and electronic screening in two-dimensional nanofluidic channels

N. Kavokine, Paul Robin, Lydéric Bocquet
The transport of fluids at the nanoscale is fundamental to manifold biological and industrial processes, ranging from neurotransmission to ultrafiltration. Yet, it is only recently that well-controlled channels with cross-sections as small as a few molecular diameters became an experimental reality. When aqueous electrolytes are confined within such channels, the Coulomb interactions between the dissolved ions are reinforced due to dielectric contrast at the channel walls: we dub this effect `interaction confinement'. Yet, no systematic way of computing these confined interactions has been proposed beyond the limiting cases of perfectly metallic or perfectly insulating channel walls. Here, we introduce a new formalism, based on the so-called surface response functions, that expresses the effective Coulomb interactions within a two-dimensional channel in terms of the wall's electronic structure, described to any desired level of precision. We use it to demonstrate that in few-nanometer-wide channels, the ionic interactions can be tuned by the wall material's screening length. We illustrate this approach by implementing these interactions in brownian dynamics simulations of a strongly confined electrolyte, and show that the resulting ionic conduction can be adjusted between Ohm's law and a Wien effect behavior. Our results provide a quantitative approach to tuning nanoscale ion transport through the electronic properties of the channel wall material.
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Extensive analysis of mitochondrial DNA quantity and sequence variation in human cumulus cells and assisted reproduction outcomes

Kishlay Kumar, Marta Venturas, D. Needleman, et al.

Are relative mitochondrial DNA (mtDNA) content and mitochondrial genome (mtGenome) variants in human cumulus cells (CCs) associated with oocyte reproductive potential and assisted reproductive technology (ART) outcomes? Neither the CC mtDNA quantity nor the presence of specific mtDNA genetic variants was associated with ART outcomes, although associations with patient body mass index (BMI) were detected, and the total number of oocytes retrieved differed between major mitochondrial haplogroups.

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Frequency splitting of chiral phonons from broken time reversal symmetry in CrI

J. Bonini, S. Ren, D. Vanderbilt, Massimiliano Stengel, C. Dreyer, Sinisa Coh

Conventional approaches for lattice dynamics based on static interatomic forces do not fully account for the effects of time-reversal-symmetry breaking in magnetic systems. Recent approaches to rectify this involve incorporating the first-order change in forces with atomic velocities under the assumption of adiabatic separation of electronic and nuclear degrees of freedom. In this work, we develop a first-principles method to calculate this velocity-force coupling in extended solids, and show via the example of ferromagnetic CrI

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The Oscura Experiment

Alexis Aguilar-Arevalo, Fabricio Alcalde Bessia, Nicolas Avalos, Daniel Baxter, Xavier Bertou, Carla Bonifazi, Ana Botti, Mariano Cababie, Gustavo Cancelo, Brenda Aurea Cervantes-Vergara, Nuria Castello-Mor, Alvaro Chavarria, Claudio R. Chavez, Fernando Chierchie, Juan Manuel De Egea, Juan Carlos D`Olivo, C. Dreyer, et all

The Oscura experiment will lead the search for low-mass dark matter particles using a very large array of novel silicon Charge Coupled Devices (CCDs) with a threshold of two electrons and with a total exposure of 30 kg-yr. The R&D effort, which began in FY20, is currently entering the design phase with the goal of being ready to start construction in late 2024. Oscura will have unprecedented sensitivity to sub-GeV dark matter particles that interact with electrons, probing dark matter-electron scattering for masses down to 500 keV and dark matter being absorbed by electrons for masses down to 1 eV. The Oscura R&D effort has made some significant progress on the main technical challenges of the experiment, of which the most significant are engaging new foundries for the fabrication of the CCD sensors, developing a cold readout solution, and understanding the experimental backgrounds.

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Higher-Order Nodal Hinge States in Doped Superconducting Topological Insulator

Sayed Ali Akbar Ghorashi, J. Cano, Enrico Rossi, Taylor L. Hughes
Doped strong topological insulators are one of the most promising candidates to realize a fully gapped three-dimensional topological superconductor (TSC). In this letter, we revisit this system and reveal a possibility for higher-order topology which was previously missed. We find that over a finite-range of doping, the Fu-Berg superconducting pairing can give rise to both Majorana surface states, and nodal hinge states. Interestingly, we observe the coexistence of surface and hinge modes in the superconducting state only when there are both bulk and surface Fermi-surfaces in the normal state. Also, we find that the hinge modes can appear for normal states consisting of doped strong or weak topological insulators. In summary, this work may allow for the discovery of superconducting hinge modes in a well explored class of materials, i.e., doped strong or weak topological insulators.
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Extracting Off-Diagonal Order from Diagonal Basis Measurements

B. Xiao, Javier Robledo Moreno, M. Fishman, D. Sels, Ehsan Khatami, Richard Scalettar
Quantum gas microscopy has developed into a powerful tool to explore strongly correlated quantum systems. However, discerning phases with topological or off-diagonal long range order requires the ability to extract these correlations from site-resolved measurements. Here, we show that a multi-scale complexity measure can pinpoint the transition to and from the bond ordered wave phase of the one-dimensional extended Hubbard model with an off-diagonal order parameter, sandwiched between diagonal charge and spin density wave phases, using only diagonal descriptors. We study the model directly in the thermodynamic limit using the recently developed variational uniform matrix product states algorithm, and draw our samples from degenerate ground states related by global spin rotations, emulating the projective measurements that are accessible in experiments. Our results will have important implications for the study of exotic phases using optical lattice experiments.
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TMDs as a platform for spin liquid physics: A strong coupling study of twisted bilayer WSe

D. Kiese, Yuchi He, Ciarán Hickey, A. Rubio, Dante M. Kennes
The advent of twisted moiré heterostructures as a playground for strongly correlated electron physics has led to a plethora of experimental and theoretical efforts seeking to unravel the nature of the emergent superconducting and insulating states. Amongst these layered compositions of two dimensional materials, transition metal dichalcogenides (TMDs) are by now appreciated as highly-tunable platforms to simulate reinforced electronic interactions in the presence of low-energy bands with almost negligible bandwidth. Here, we focus on the twisted homobilayer WSe
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